Download | - View final version: Nanocomposites of graphene oxide, Ag nanoparticles, and magnetic ferrite nanoparticles for elemental mercury (Hg0) removal (PDF, 1.2 MiB)
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DOI | Resolve DOI: https://doi.org/10.1039/C4RA16016A |
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Author | Search for: Liu, Yuxi; Search for: Tian, Chong; Search for: Yan, Bin; Search for: Lu, Qingye; Search for: Xie, Yijun; Search for: Chen, Jian1; Search for: Gupta, Rajender; Search for: Xu, Zhenghe; Search for: Kuznicki, Steven M.; Search for: Liu, Qingxia; Search for: Zeng, Hongbo |
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Affiliation | - National Research Council of Canada. National Institute for Nanotechnology
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Format | Text, Article |
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Abstract | Mercury emission from combustion flue gas causes considerable environmental challenges and serious adverse health threats, and elemental mercury (Hg0) is the most challenging chemical form for removal. In this work, four types of graphene oxide (GO) based composite adsorbents were successfully synthesized by depositing Ag nanoparticles (NPs) and/or magnetic ferrite NPs on GO sheets (denoted as GO, GO–Ag, MGO and MGO–Ag), characterized and applied for the removal of Hg0 for the first time. The presence of Ag NPs on GO greatly enhances the Hg0 removal capability of GO–Ag and MGO–Ag as compared to that of pure GO, which is mainly attributed to the amalgamation of Hg0 on Ag NPs. MGO–Ag shows the best Hg0 removal performance and thermal tolerance among the four types of adsorbents developed, which can effectively capture Hg0 up to 150–200 °C in a simulated flue gas environment and can be also effectively recycled and reused. Our results indicate that the graphene oxide based composites (i.e. MGO–Ag) have significant potential applications for mercury emission control in coal-fired power plants. |
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Publication date | 2015-01-27 |
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Publisher | Royal Society of Chemistry |
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In | |
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Language | English |
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Peer reviewed | Yes |
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NPARC number | 23001565 |
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Export citation | Export as RIS |
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Report a correction | Report a correction (opens in a new tab) |
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Record identifier | 3ad27da5-41b3-490a-9f79-95c9fb750232 |
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Record created | 2017-03-07 |
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Record modified | 2020-05-30 |
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