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In Situ Visualization of Drop Deformation, Erosion, and Breakup in High Viscosity Ratio Polymeric Systems Under High Shearing Stress Conditions

Par Conseil national de recherches du Canada

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DOITrouver le DOI : https://doi.org/10.1002/app.22744
AuteurRechercher : ; Rechercher : 1
Affiliation
  1. Conseil national de recherches du Canada. Institut des matériaux industriels du CNRC
FormatTexte, Article
ISSN1097-4628
0021-8995
Sujetshearing flow visualization; high viscosity ratio; drop deformation; drop breakup; dispersion by surface erosion mechanism
Résumé
In this paper, deformation and breakup under simple shear of single molten polymer drops in a polymer matrix were investigated. Flow visualization was carried out in a Couette-Flow apparatus under relatively high shear rates and temperatures up to 230°C. Drop/Matrix combinations were composed of polystyrene drops of 0.5– 0.6 mm in diameter in polyethylene matrix, and ethylene– propylene copolymer drops of approximately the same size in polypropylene matrix. The deformation and breakup processes were studied under steady state and time-dependent shearing conditions. Either for steady state or time-dependant shearing conditions, drop elasticity generated at relatively high shear rates helped the drops to align perpendicular to the flow direction, i.e., parallel to vorticity axis. Also, the most striking non-Newtonian effects for the high viscosity ratio systems were the surface erosion and the drop splitting mechanisms. The particles eroded off the main droplet surface were very fine, in the range of 10–50 m, and led to a significant reduction in main drop size before its final breakup.
Date de publication
Dans
  • Journal of Applied Polymer Science 100, nº 4 (1 janvier 2006) : 2582–2591.
Langueanglais
Publications évaluées par des pairsOui
Numéro du CNRCNRCC 53753
Numéro NPARC15930970
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Identificateur de l’enregistrement30102174-cf7a-44e3-b76d-ae78e0aae419
Enregistrement créé2010-08-17
Enregistrement modifié2020-04-22
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