| DOI | Trouver le DOI : https://doi.org/10.1103/PhysRevLett.98.187402 |
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| Auteur | Rechercher : Dietzek, Benjamin; Rechercher : Gräfe, Stefanie1; Rechercher : Schmitt, Michael; Rechercher : Yartsev, Arkady; Rechercher : Pascher, Torbjörn; Rechercher : Sundström, Villy; Rechercher : Kiefer, Wolfgang; Rechercher : Ivanov, Misha Yu1 |
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| Affiliation | - Conseil national de recherches du Canada. Institut Steacie des sciences moléculaires du CNRC
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| Format | Texte, Article |
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| Sujet | dielectric materials; optical phase matching; stimulated Raman scattering; vibrational modes |
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| Résumé | We use high-order Raman scattering in a bulk dielectric to characterize coherent dynamics with precision typical for gas phase experiments. The experimental pump-probe approach allows for the simultaneous observation and separation in space and time of the individual contributions of different-order Raman processes to a coherent wave packet without relying on phase-matching conditions and within the same experimental geometry. We propose a novel technique to discriminate between stimulated excitation of vibronic levels in the impulsive and intermediate excitation regimes, futhermore allowing us to distinguish between different pathways contributing to the same fifth-order Raman processes. |
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| Date de publication | 2007-05-04 |
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| Dans | |
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| Langue | anglais |
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| Numéro NPARC | 12339117 |
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| Exporter la notice | Exporter en format RIS |
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| Signaler une correction | Signaler une correction (s'ouvre dans un nouvel onglet) |
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| Identificateur de l’enregistrement | 3e55f85b-9468-484b-ac6b-c6208ba9c017 |
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| Enregistrement créé | 2009-09-11 |
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| Enregistrement modifié | 2020-05-10 |
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