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Time-resolved photoelectron angular distributions: concepts, applications, and directions

Par Conseil national de recherches du Canada

DOITrouver le DOI : https://doi.org/10.1146/annurev.physchem.53.082101.130051
AuteurRechercher : 1
Affiliation
  1. Conseil national de recherches du Canada. Institut Steacie des sciences moléculaires du CNRC
FormatTexte, Article
Sujetfemtochemistry; angle-resolved photoionization; photoelectron imaging; radiationless transitions; time-dependent alignment
Résumé
The use of photoelectron angular distributions (PADs) as a probe in short-pulse, pump-probe scenarios is reviewed. We focus on concepts, on the insight that can be gained through theoretical analysis, on applications, and on future opportunities. Time-resolved PADs are sensitive to both the time-evolving rotational composition of wavepackets and their time-evolving electronic symmetry. The former feature renders this observable a potential probe of molecular structure, intensity effects, and rotational perturbations. The latter feature renders the PAD a potential probe of radiationless transitions.
Date de publication
Dans
  • Annual Review of Physical Chemistry 53 (28 novembre 2003) : 41–65.
Numéro NPARC12327058
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Identificateur de l’enregistrement8991736b-92f2-48d1-81d0-3c5ffe893be9
Enregistrement créé2009-09-10
Enregistrement modifié2020-04-02
Date de modification :