| Téléchargement | - Voir la version finale : Nonlinear enhancement of radiative absorption by black carbon in response to particle mixing structure (PDF, 1.6 Mio)
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| DOI | Trouver le DOI : https://doi.org/10.1029/2021GL096437 |
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| Auteur | Rechercher : Wang, YuanyuanIdentifiant ORCID : https://orcid.org/0000-0003-4190-6418; Rechercher : Li, WeijunIdentifiant ORCID : https://orcid.org/0000-0003-4887-4260; Rechercher : Huang, Jin; Rechercher : Liu, LeiIdentifiant ORCID : https://orcid.org/0000-0002-7171-1454; Rechercher : Pang, Yuner; Rechercher : He, CenlinIdentifiant ORCID : https://orcid.org/0000-0002-7367-2815; Rechercher : Liu, Fengshan1; Rechercher : Liu, DantongIdentifiant ORCID : https://orcid.org/0000-0003-3768-1770; Rechercher : Bi, LeiIdentifiant ORCID : https://orcid.org/0000-0002-1996-880X; Rechercher : Zhang, Xiaoye; Rechercher : Shi, ZongboIdentifiant ORCID : https://orcid.org/0000-0002-7157-543X |
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| Affiliation | - Conseil national de recherches Canada. Centre de recherche en métrologie
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| Bailleur de fonds | Rechercher : National Natural Science Foundation of China |
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| Format | Texte, Article |
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| Résumé | Black carbon (BC) strongly absorbs solar radiation, contributing to global warming. Absorption enhancement of BC particles is difficult to quantify due to an inadequate representation of their complex morphology and mixing structures, as well as interaction with radiation. Here, we apply a 3D method accounting for detailed BC mixing structures to predict the absorption enhancement of individual BC particles (Eabs) and the total BC particle population (Eabs, bulk). The diverse range of mixing structures in individual BC particles leads to variable Eabs that could hardly be predicted by empirical approximations. We find that the volume proportion of the BC embedded in coating (F) determines Eabs when the particle to BC core diameter ratio (Dₚ/D꜀) is larger than 2.0. Our findings reveal the potential mechanism behind the differences in observed and modeled Eabs, bulk. The framework builds a bridge connecting the microscopic mixing structure of individual BC particle with Eabs, bulk. |
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| Date de publication | 2021-12-13 |
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| Maison d’édition | Wiley
American Geophysical Union |
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| Licence | |
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| Dans | |
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| Langue | anglais |
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| Publications évaluées par des pairs | Oui |
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| Exporter la notice | Exporter en format RIS |
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| Signaler une correction | Signaler une correction (s'ouvre dans un nouvel onglet) |
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| Identificateur de l’enregistrement | 99dae84a-3197-4bf8-8732-cacc6570ba52 |
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| Enregistrement créé | 2023-02-20 |
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| Enregistrement modifié | 2023-02-21 |
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