| DOI | Trouver le DOI : https://doi.org/10.1073/pnas.0907434106 |
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| Auteur | Rechercher : Smirnova, Olga1; Rechercher : Patchkovskii, Serguei1; Rechercher : Mairesse, Yann1; Rechercher : Dudovich, Nirit1; Rechercher : Ivanov, Misha Yu1 |
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| Affiliation | - Conseil national de recherches du Canada
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| Format | Texte, Article |
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| Sujet | molecular structures; electrons; strong field ionization; multielectron dynamics; high harmonic generation; multielectron dynamics; strong-field ionization |
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| Résumé | Molecular structures, dynamics and chemical properties are determined by shared electrons in valence shells. We show how one can selectively remove a valence electron from either ∥ vs. ∑ or bonding vs. nonbonding orbital by applying an intense infrared laser field to an ensemble of aligned molecules. In molecules, such ionization often induces multielectron dynamics on the attosecond time scale. Ionizing laser field also allows one to record and reconstruct these dynamics with attosecond temporal and sub-Ångstrom spatial resolution. Reconstruction relies on monitoring and controlling high-frequency emission produced when the liberated electron recombines with the valence shell hole created by ionization. |
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| Date de publication | 2009-09-29 |
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| Dans | |
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| Langue | anglais |
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| Publications évaluées par des pairs | Oui |
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| Numéro NPARC | 15073184 |
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| Exporter la notice | Exporter en format RIS |
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| Signaler une correction | Signaler une correction (s'ouvre dans un nouvel onglet) |
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| Identificateur de l’enregistrement | a4971da6-0cc7-44c9-8104-70cdc78ae00c |
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| Enregistrement créé | 2010-05-03 |
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| Enregistrement modifié | 2020-04-16 |
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